Laser-controlled fluorescence in two-level systems.

نویسندگان

  • Jamie M Leeder
  • David S Bradshaw
  • David L Andrews
چکیده

The ability to modify the character of fluorescent emission by a laser-controlled, optically nonlinear process has recently been shown theoretically feasible, and several possible applications have already been identified. In operation, a pulse of off-resonant probe laser beam, of sufficient intensity, is applied to a system exhibiting fluorescence, during the interval of excited-state decay following the initial excitation. The result is a rate of decay that can be controllably modified, the associated changes in fluorescence behavior affording new, chemically specific information. In this paper, a two-level emission model is employed in the further analysis of this all-optical process; the results should prove especially relevant to the analysis and imaging of physical systems employing fluorescent markers, these ranging from quantum dots to green fluorescence protein. Expressions are presented for the laser-controlled fluorescence anisotropy exhibited by samples in which the fluorophores are randomly oriented. It is also shown that, in systems with suitably configured electronic levels and symmetry properties, fluorescence emission can be produced from energy levels that would normally decay nonradiatively.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Mixing of the Immiscible Liquids in the Entrance Region of a T-Type Chamber Using Laser Induced Fluorescence (LIF) Method

A Laser Induced Fluorescence technique (LIF) has been used to study the mixing behavior of two emerging streams in a T-Type mixing chamber. A mixing index on the basis of digital image light intensities is calculated. It has been shown that averaging over more than 800 images leads to a stable mixing index calculation. Moreover, the effect of equal and un-equal flow rates on the mixing behavior...

متن کامل

Effect of Low-Level Laser Therapy on Muscle Strength and Endurance and Post-Exercise Recovery of Young Adult: A Double-Blind, Placebo-Controlled, Randomized Clinical Trial

Background. Recovery or post-exercise rehabilitation is an essential part of exercise training. Low-level Laser Therapy (LLLT) is a modality increasing interest for recovery because of having a conservative and non-aggressive method. LLLT also decreases the production of fatigue-related biomechanical markers, such as lactate, C-reactive protein (CRP), and Creatine kinase (CK). Objectives. To i...

متن کامل

LASERS WITHOUT INVERSION: DENSITY OPERATOR METHOD

A quantum theory of a two and three-level laser with injected atomic coherence is developed by using a density operator method, to the best of our knowledge, for the first time. The initial atomic coherence plays an essential role. At steady state, the equation of motion for the density operator yields to exhibit laser without inversion and a phase locking but no threshold for the laser fie...

متن کامل

Time-resolved two-dimensional imaging of ground-state species using laser-induced fluorescence

Time-resolved two-dimensional imaging of ground-state species using laser-induced fluorescence" (1983). Laser-induced fluorescence has been employed to obtain two-dimensional images of the spatial distribution of a vapor in the ground state with nanosecond resolution. The method has a wide range of potential applications, as it can be used to observe any species which has energy levels accessib...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:
  • The journal of physical chemistry. B

دوره 115 18  شماره 

صفحات  -

تاریخ انتشار 2011